硫化物钝化对InAs纳米线光学特性的影响
作者:
作者单位:

1.上海理工大学 材料科学与工程学院,上海 200093;2.中国科学院上海技术物理研究所 红外物理国家重点实验室,上海 200083

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中图分类号:

TN304.2

基金项目:

国家自然科学基金 11874377;上海市自然科学基金 18ZR1445700国家自然科学基金(11874377);上海市自然科学基金(18ZR1445700)


The influence of sulfide passivation on optical properties of InAs nanowires
Author:
Affiliation:

1.School of Materials Science and Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China;2.State Key Laboratory of Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, Shanghai 200083, China

Fund Project:

the National Natural Science Foundation of China 11874377;the Natural Science Foundation of Shanghai 18ZR1445700Supported by the National Natural Science Foundation of China (11874377); the Natural Science Foundation of Shanghai (18ZR1445700)

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    摘要:

    针对InAs纳米线表面氧化造成的发光效率低的问题,采用十八硫醇和硫化铵钝化了由化学气相沉积设备生长的闪锌矿结构的InAs纳米线。对硫化物钝化前后的InAs纳米线进行温度依赖的光致发光光谱测试。实验结果表明,十八硫醇和硫化铵钝化的InAs纳米线在25 K温度下的发光效率与未钝化的InAs纳米线相比分别提高了~ 6倍和~7倍,此外,可以在室温下探测到硫化铵钝化的InAs纳米线的光致发光,这为未来基于InAs纳米线的中红外纳米光子器件提供了可能性。

    Abstract:

    To solve the problem of low luminescence efficiency caused by the surface oxidation of InAs nanowires, C18H38S and (NH4)2S were adopted to passivate zinc blende (ZB) InAs nanowires synthesized by chemical vapor deposition (CVD). Photoluminescence (PL) spectra of (before and after sulfide passivation) InAs nanowires were performed. The experimental results show that the PL emission efficiency of C18H38S and (NH4)2S passivated InAs nanowires are ~ 6 times and ~ 7 times higher than that of unpassivated InAs nanowires at 25 K, respectively, in addition, the PL of (NH4)2S passivation InAs nanowires is detected at room temperature, which provides a possibility for future InAs nanowires based middle infrared nanophoton devices.

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李宝宝,李生娟,陈刚,李世民,王兴军.硫化物钝化对InAs纳米线光学特性的影响[J].红外与毫米波学报,2019,38(5):591~597]. LI Bao-Bao, LI Sheng-Juan, CHEN Gang, LI Shi-Min, WANG Xing-Jun. The influence of sulfide passivation on optical properties of InAs nanowires[J]. J. Infrared Millim. Waves,2019,38(5):591~597.]

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  • 收稿日期:2019-03-18
  • 最后修改日期:2019-07-02
  • 录用日期:2019-04-17
  • 在线发布日期: 2019-08-31
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