Broadband and high-sensitivity cavity-enhanced dual-comb spectroscopy for gas absorption measurements
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1Zhejiang Key Laboratory of Quantum State Control and Optical Field Manipulation, School of Information Science and Engineering, Zhejiang Sci-Tech University, Hangzhou, 310018, China;2State Key Laboratory of Precision Measurement Technology and Instruments, Department of Precision Instrument, Tsinghua University, Beijing, 100084, China

Clc Number:

O433.1

Fund Project:

Supported by the National Natural Science Foundation of China (62275138, 62271449), the Fundamental Research Funds of Zhejiang Sci-Tech University (25222174-Y)

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    Abstract:

    This work investigates the impact of cavity mirror parameters on the transmission bandwidth and sensitivity of cavity-enhanced dual-comb spectroscopy (CE-DCS) systems, starting from the principle of cavity-comb coupling. A comprehensive evaluation metric for cavity mirror performance is proposed. Based on this metric, a low-dispersion cavity mirror with a finesse of 15,000 was designed and fabricated. A CE-DCS system was developed using the designed mirror. Absorption spectroscopy experiments were conducted for CO2 gas, and the results show that the system achieved a transmission bandwidth of 370 cm-1 (88 % of the original comb spectrum), with a noise-equivalent absorption (NEA) of 1.45×10-10 cm-1Hz-1. These results validate the accuracy and effectiveness of the designed mirror in achieving broadband and high-sensitivity gas absorption spectroscopy measurements, providing a solid technical foundation for trace gas quantitative analysis.

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History
  • Received:August 28,2025
  • Revised:October 22,2025
  • Adopted:January 08,2026
  • Online: April 24,2026
  • Published:
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