宽带、高灵敏腔增强双光梳气体吸收光谱测量技术研究
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作者单位:

1浙江理工大学 信息科学与工程学院 全省量子物态与光场调控重点实验室, 浙江 杭州 310018;2清华大学 精密仪器系 精密测试技术及仪器全国重点实验室, 北京 100084

作者简介:

E-mail:zhanglieshan@zstu.edu.cn

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中图分类号:

O433.1

基金项目:

国家自然科学基金(62275138,62271449),浙江理工大学基本科研业务费专项(25222174-Y)


Broadband and high-sensitivity cavity-enhanced dual-comb spectroscopy for gas absorption measurements
Author:
Affiliation:

1Zhejiang Key Laboratory of Quantum State Control and Optical Field Manipulation, School of Information Science and Engineering, Zhejiang Sci-Tech University, Hangzhou 310018, China;2State Key Laboratory of Precision Measurement Technology and Instruments, Department of Precision Instrument, Tsinghua University, Beijing 100084, China

Fund Project:

Supported by the National Natural Science Foundation of China (62275138, 62271449), the Fundamental Research Funds of Zhejiang Sci-Tech University (25222174-Y)

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    摘要:

    从腔梳耦合原理出发研究了腔增强双光梳光谱(CE-DCS)测量系统中腔镜参数对透射带宽和灵敏度的影响,提出了腔镜参数综合评价指标。根据该指标设计并加工了一款具备低色散属性,精细度为15 000的腔镜,在此基础上开发了一套CE-DCS系统。对CO<sub>2</sub>气体进行了吸收光谱测量实验,结果表明该系统实现了370 cm<sup>-1</sup>的透射带宽(原始梳谱利用率达88 %),噪声等效吸收系数为1.45×10<sup>-10</sup> cm<sup>-1</sup>Hz<sup>-1</sup>。验证了所设计腔镜及系统在气体吸收光谱测量方面的准确性和有效性,并为痕量气体定量分析等应用提供了技术支撑。

    Abstract:

    This work investigates the impact of cavity mirror parameters on the transmission bandwidth and sensitivity of cavity-enhanced dual-comb spectroscopy (CE-DCS) systems, starting from the principle of cavity-comb coupling. A comprehensive evaluation metric for cavity mirror performance is proposed. Based on this metric, a low-dispersion cavity mirror with a finesse of 15,000 was designed and fabricated. A CE-DCS system was developed using the designed mirror. Absorption spectroscopy experiments were conducted for CO<sub>2</sub> gas, and the results show that the system achieved a transmission bandwidth of 370 cm<sup>-1</sup> (88 % of the original comb spectrum), with a noise-equivalent absorption (NEA) of 1.45×10<sup>-10</sup> cm<sup>-1</sup>Hz<sup>-1</sup>. These results validate the accuracy and effectiveness of the designed mirror in achieving broadband and high-sensitivity gas absorption spectroscopy measurements, providing a solid technical foundation for trace gas quantitative analysis.

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  • 收稿日期:2025-08-28
  • 最后修改日期:2026-07-23
  • 录用日期:2026-01-08
  • 在线发布日期: 2026-07-16
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